Universal thermal breakdown of polaron coherence in one, two, and three dimensions

Abstract

How a polaron loses its quasiparticle coherence with increasing temperature is a long-standing open problem. Holstein addressed it in 1959 only in the extreme antiadiabatic, strong-coupling limit, while more recent numerically exact approaches are largely restricted to one dimension. Here we solve this problem on square and simple cubic lattices across the weak-, intermediate-, and strong-coupling regimes. We show that the polaron effective mass $m^{\ast }$ and inverse lifetime $1/\tau$ increase monotonically with temperature until, at $T\sim 0.5\Omega$, the quasiparticle peak dissolves into a broad incoherent thermal continuum. The phonon frequency $\Omega$ therefore defines a universal coherence scale, independent of dimensionality and coupling strength, validating Holstein's prediction far beyond the regime in which it was derived. These results follow from a finite-temperature generalization of the Momentum Average (MA) approximation, yielding a closed-form, diagrammatically derived self-energy that is asymptotically exact in the strong-coupling limit at all temperatures. Benchmark comparisons demonstrate excellent quantitative agreement of the resulting 1D spectral functions with the numerically exact Variational Exact Diagonalization-Finite-Temperature Lanczos Method (VED-FTLM) and finite-$T$ Density Matrix Renormalization Group (DMRG).

8 pages, 5 figures (main text, including End Matter); Supplemental Material: 14 pages, 17 figures. Dataset available at https://doi.org/10.5683/SP4/LYHBP7