Localizing polymers promotes the centre-mode elastic instability

Abstract

The centre-mode elastic instability, prevalent in rectilinear flows of dilute polymer solutions, allows dynamic states to emerge even in the absence of inertia. Here, we show that this instability can be significantly enhanced when the base flow has a nonuniform spatial-distribution of polymers. In such a flow, the polymeric stress not only depends on the conformation tensor (determined here by the Oldroyd-B equation) but also varies proportionally with the polymer concentration field, which satisfies a scalar transport equation. Focusing on the inertialess Stokes limit, we first consider the simple setting of periodic Kolmogorov flow. A linear stability analysis shows that a nonuniform polymer concentration either promotes or suppresses the centre-mode instability, depending on whether the polymers are localised near or away from the maximum of the base-velocity profile. We then focus on a base flow with a distinct polymer-laden stream overlying the base-velocity maximum, and sandwiched between polymer-free streams. We find that the critical Weissenberg number (product of the elastic relaxation time and the typical strain-rate) at the onset of instability undergoes a sudden decrease as the total polymer loading is increased. An energy analysis attributes this destabilisation to elastic feedback forces that arise from concentration gradients near the interfaces between the polymer-laden and polymer-free streams. The insights from Kolmogorov flow are shown to carry over to channel flow, where localising polymers about the centreline strongly promotes the centre-mode instability.

23 pages, 15 figures