Vector-field control and emergent basal-plane anisotropy of magnetic textures in noncentrosymmetric (Fe${}_{0.63}$Ni${}_{0.3}$Pd${}_{0.07}$)${}_3$P

Abstract

(Fe${}_{0.63}$Ni${}_{0.3}$Pd${}_{0.07}$)${}_3$P is a room-temperature magnet with $S_4$ symmetry that hosts a rich variety of topological spin textures. Here, we report a combined resonant small-angle x-ray scattering and ptychography study of (Fe${}_{0.63}$Ni${}_{0.3}$Pd${}_{0.07}$)${}_3$P in vector magnetic fields over a broad temperature range. We demonstrate deterministic vector-field control of magnetic stripe domains, where in-plane fields continuously rotate their orientation via a transition from a chiral stripe to an achiral fan configuration. Furthermore, at 50 K and below, the stripe orientation becomes metastably pinned and retains its field-trained direction. While the magnitude of the wavevector is nearly isotropic within the basal plane at room temperature, a pronounced temperature evolution of anisotropic interactions emerges upon cooling. In particular, non-trivial anisotropy axes develop at 20-50 K reflecting the combined effects of magnetocrystalline anisotropy, anisotropic exchange, and Dzyaloshinskii-Moriya interaction (DMI), whose effective orientation is found to rotate with temperature. These results establish (Fe${}_{0.63}$Ni${}_{0.3}$Pd${}_{0.07}$)${}_3$P as a model system for vector-field control of chiral spin textures and reveal a previously unrecognized temperature-driven evolution of the effective DMI landscape in a noncentrosymmetric magnet.