Effect of pressure on the magnetic properties of (Co${}_{0.5}$Fe${}_{0.5}$)${}_5$GeTe${}_2$

Abstract

Cobalt-doped Fe${}_5$GeTe${}_2$ possesses a rich magnetic phase diagram as a function of Co concentration. The nature of magnetic order in (Co${}_{0.5}$Fe${}_{0.5}$)${}_5$GeTe${}_2$ is especially interesting, as it has been shown to exhibit ferromagnetic order, A-type antiferromagnetic (AFM) order, or potentially both at the same time. Here we present magnetoresistance measurements on antiferromagnetic (Co${}_{0.5}$Fe${}_{0.5}$)${}_5$GeTe${}_2$ at a series of pressures and extract the anisotropy and interlayer exchange fields using the two-sublattice model. We show a 50 % increase of the interlayer exchange at 2 GPa, highlighting the sensitivity of magnetic properties to interlayer distance. In addition, we find that the sharp hysteretic transitions observed within the AFM state can be qualitatively described by a linear chain model, which suggests an even-odd effect as a function of layer number instead of a coexisting ferromagnetic phase.