Revealing quantum geometry effects in magic angle twisted bilayer graphene using the circular photogalvanic effect

Abstract

We report a photocurrent studies of a magic angle twisted bilayer graphene device using near infrared light. Through photocurrent imaging and polarization dependence, we separate the photo-thermoelectric effect from the photogalvanic effect. We observe a circular photogalvanic effect (CPGE) over a wide range of doping and temperature. The CPGE at normal incidence constraints the symmetry of the system to C${}_1$, and points to a Berry curvature dipole, in agreement with theoretical predictions for strained graphene. Remarkably, the CPGE vanishes for filling $-2.5<\hat{I}½<-1.5$, suggesting an additional symmetry breaking in that regime. Insight into this effect is obtained through Berry curvature dipole calculations, which emphasize a novel symmetry breaking effect near $\hat{I}½=-2$.

Includes Supplemental Material