Zero-Field Thermal Hall Effect in Insulator

Abstract

Fourier's law dictates that heat flow is usually parallel to the applied temperature gradient. However, under a high magnetic field, heat flow carried by both electrons in conductors and phonons in insulators can be deflected, a phenomenon known as thermal Hall effect. Intriguingly, we observe at zero field a spontaneous thermal Hall effect in an antiferromagnetic insulator. Despite a vanishingly small uncompensated magnetization, the magnitude of this effect is surprisingly large, comparable to typical responses induced by several teslas of external field. This zero-field behavior indicates that charge-neutral heat carriers can be governed by an intrinsic effective field arising from the unique spin arrangement. Our discovery challenges the centuries-old preconception of heat conduction and open up new avenues for exploring non-trivial topological responses in quantum materials.