Revealing Hund superdispersion with tunneling spectroscopy

Abstract

In cuprate superconductors, electron-electron repulsion results in characteristic spectroscopic features known as `waterfalls', where the sharp quasiparticle dispersion transitions into broad Hubbard bands. However, in multi-orbital systems, the additional Hund coupling results in behavior that defies the conventional Mott--Hubbard paradigm, creating qualitatively distinct `superdispersive' features in the spectral function. Here, we use tunneling spectroscopy to reveal this signature of Hund physics in Sr${}_2$RuO${}_4$. By combining density functional theory, dynamical mean-field theory, and continuum local density of states calculations, we show that the experimental features are in excellent agreement with theoretical predictions and intimately linked to the non-monotonous energy dependence of the real part of the self-energy in a Hund metal. Our results provide direct experimental evidence for Hund-induced spectroscopic features and open a new route to probing correlation effects in quantum materials.

29 pages including supplementary material, 4 figures in main text plus 2 supplementary figures