Chirality and quasi-long-range order in finite-flux Gutzwiller states for magnetized frustrated magnets

Abstract

We study Gutzwiller-projected wavefunctions for triangular-lattice U(1) Dirac spin liquids in a Zeeman field, where we allow the U(1) gauge field to develop a gauge flux, resulting in (spin-split) spinon Landau levels. We find that at a given magnetization, the optimal candidate state has a finite flux chosen such that the spinon filling lies in a $|C|=1$ Landau-level gap: it gives the lowest variational energy and the smallest energy variance within our correlation-matrix reconstruction for local Heisenberg-type models. By symmetry, we argue that the finite gauge flux results in a non-zero (staggered) scalar spin chirality, as also numerically observed, and further find that the $|C|=1$ state exhibits dominant quasi-long-ranged $120^{\circ }$ magnetic correlations. Studying the next-to-optimal wavefunction with a $|C|=2$ Landau-level gap, we observe unusual spin-nematic correlations. Our results may provide guidance for analyzing the magnetic-field response of DSL candidate materials and offer numerical diagnostics that can connect to the underlying theory of spinons coupled to an emergent U(1) gauge field.

9 pages, 7 figures; Supplementary Materials: 13 pages