Viewpoint: On the Emergence of van der Waals Magnets: A Personal Reflection

Abstract

The observation of magnetism in atomically thin van der Waals (vdW) antiferromagnets (FePS${}_3$, NiPS${}_3$, and MnPS${}_3$) in 2016 marked an important moment in the development of two-dimensional (2D) physics. In this personal reflection, I describe how a simple question, posed in the early 2010s, motivated experimental efforts that culminated in the demonstration of antiferromagnetic order in monolayer FePS${}_3$. Alongside subsequent reports of vdW ferromagnets in 2017, these developments helped establish intrinsic magnetism as a viable degree of freedom in atomically thin materials. I close with personal lessons drawn from this period and a perspective on the opportunities that now shape the field's second decade and beyond.

J. Phys. Condens. Matter (in press)