Many-electron characterizations of higher-charge superconductors

Abstract

The theoretical understanding of conventional superconductivity as the phonon-assisted formation and condensation of two-electron Cooper pairs is a significant triumph in condensed matter physics. Here, we propose many-electron characterizations of higher-charge superconductivity with Cooper pairs consisting of more than two electrons, by implementing translation symmetrization on parent pair-density-wave-ordered states. In particular, we demonstrate many-electron constructions with vanishing charge-2$e$ sectors, but with sharp signatures in charge-$4e$ or charge-$6e$ expectation values instead. Such characterizations are consistent with previous phenomenology of vestigial order and Ginzburg-Landau theory. Furthermore, we demonstrate that at the microscopic level, momentum conservation alone may be vital and sufficient for the robust emergence of higher-charge superconductivity. Our study thus offers a novel, general, and microscopic route to understand and characterize higher-charge superconductivity, including nontrivial experimental signatures such as fractional magnetic flux and period in interferometry, as well as localized Cooper pairs at lattice topological defects.

arXiv comment8 pages, 5 figures