Microscopic Model of Exciton Polarons in 2D Wigner Crystals

Abstract

Monolayer transition-metal dichalcogenides (TMDs) provide a platform for realizing Wigner crystals and enable their detection via exciton spectroscopy. We develop a microscopic theoretical model for excitons interacting with the localized electrons of the Wigner crystal, including their vibrational motion. In addition to the previously observed exciton-Umklapp feature, the theory reproduces and explains the higher-band attractive-polaron resonances recently reported experimentally. Our model further uncovers that the appearance of two equal-strength and parallel attractive polarons, as commonly observed in WSe${}_2$ and WS${}_2$, is a signature of strong correlations in the electronic system. Altogether, our results demonstrate that accounting for electronic interactions is essential to reproduce and interpret the exciton-polaron spectra of TMDs.

11 pages, 8 figures