Engineering Zeeman-manifold quintets using state-dependent light shifts in neutral atoms

Abstract

We present a general method for engineering qudits through individually addressable transitions between Zeeman sublevels, achieved by combining a large linear Zeeman shift with a state-dependent light shift. This approach lifts the degeneracy between adjacent states while simultaneously tuning their energy splittings into the radio-frequency (RF) domain, enabling coherent manipulation within the Zeeman manifold using experimentally accessible drive frequencies. As a concrete realization, we investigate the implementation of an $SU(5)$ \emph{quintet} encoded in the Zeeman sublevels of the long-lived ${}^3{\mathrm{P}}_2$ state of neutral ${}^{88}\mathrm{Sr}$ atoms confined in far-detuned, $\ddot{I}{ƒ}^{-}$-polarized optical tweezers. Using realistic experimental parameters, we numerically demonstrate full control of the \emph{quintet} manifold, including initialization into a specific $SU(5)$ basis state via a multi-photon transfer, coherent state- and site-selective single-qudit rotations driven by RF fields, and fast state-selective optical readout. Our simulations predict state-preparation fidelities of $\mathcal{F}\simeq 0.99$ within $\sim 1\hat{I}¼\mathrm{s}$, single-qudit gate fidelities of $\mathcal{F}\simeq 0.99$ with $\ddot{I}€$-pulse durations of $\sim 2.5\hat{I}¼\mathrm{s}$, and fast destructive imaging with durations below $10\hat{I}¼\mathrm{s}$. These results establish a broadly applicable framework for high-fidelity control of Zeeman sublevel-encoded qudits and highlight the ${}^3{\mathrm{P}}_2$ manifold in strontium as a promising platform for scalable qudit-based quantum technologies.

18 pages, 16 figures