Measurement of the ${}^{35}Cl(n,p{)}^{35}S$ cross-section at the CERN n\_TOF facility from subthermal energy to 120 keV

Abstract

Background: The ${}^{35}Cl(n,p{)}^{35}S$ reaction is of special interest in three different applications. First, in Boron Neutron Capture Therapy due to the presence of ${}^{35}Cl$ in brain and skin tissue. Second, it is involved in the creation of ${}^{36}S$, whose astrophysical origin remains unresolved. Third, in the designing of fast nuclear reactors of new generation based on molten salts. Purpose: To measure the ${}^{35}Cl(n,p{)}^{35}S$ cross-section from thermal energy to 120 keV, determine the resonance parameters in this range and Maxwellian Averaged Cross-Section (MACS). Method: We made use of the Time-of-Flight technique with microMEGAS detectors at Experimental Area 2 (EAR-2) of n\_TOF facility at CERN. The ${}^{10}B(n,\hat{I}\pm {)}^{7}Li$ and ${}^{235}U(n,f)$ reactions were used as references. Rutherford Back-scattering Spectrometry technique was performed at Centro Nacional de Aceleradores (CNA) in Sevilla, in order to accurately determine the masses of the irradiated samples. Results: We obtain a thermal cross-section of $0.470\pm 0.009$ barns. The $1/v$ energy dependence of the cross-section is observed up to the first resonance at 0.398 keV, the resonances up to 120 keV are analyzed and MACS calculated for $k_{B}T$ from 1 to 100 keV. Conclusions: The ${}^{35}Cl(n,p{)}^{35}S$ cross-section has been obtained over a wide energy range for the first time, with high accuracy across the aforementioned range. The thermal cross-section and first two resonances are in agreement with latest evaluation in ENDF/B-VIII.1, while lower resonance strength was found for high energy resonances. These data are used to calculate the MACS for different $k_{B}T$.

15 pages, 13 figures, 4 tables