Kitaev-derived Gapless Spin Liquid in the $K$-$J$-$\Gamma$-${\Gamma }^{\prime }$ Quantum Magnet Na${}_2$Co${}_2$TeO${}_6$

Abstract

The realization of quantum spin liquids (QSLs) in Kitaev magnets represents an intriguing topic in frustrated quantum magnetism. Despite prediction in the pure Kitaev honeycomb model, realization of QSLs in realistic systems and materials remain scarce. The recent discovery of cobalt-based compound Na${}_2$Co${}_2$TeO${}_6$ has raised significant research interest. By establishing a realistic $K$-$J$-$\Gamma$-${\Gamma }^{\prime }$ model for Na${}_2$Co${}_2$TeO${}_6$ -- with a dominant antiferromagnetic (AFM) Kitaev interaction ($K>0$) that quantitatively explains its thermodynamics measurements -- we reveal an intermediate gapless QSL phase under [111] magnetic fields with tensor-network calculations. We confirm the QSL nature of this phase by demonstrating its adiabatic connection to the intensively studied intermediate QSL of the pure AFM Kitaev model under out-of-plane fields. Our results show excellent agreement with recent high-field experiments, thereby explaining the intermediate-field phase in Na${}_2$Co${}_2$TeO${}_6$. These findings bridge the gap between theoretical proposals for a Kitaev-derived QSL and experimental realization, opening new avenues for exploring exotic quantum states of matter in realistic Kitaev materials.

6 pages, 4 figures, Supplementary materials