Griffiths phases in structurally disordered CeRhSn: Experimental evidence and theoretical modeling

Abstract

Our report paves the way for insight into a structural disorder and its impact on the physical properties of strongly correlated electron systems (SCESs). In a critical regime, each perturbation, e.g., disorder due to structural defects or doping, can have a significant effect on the nature of the quantum macrostate of these materials. For a select group of SCESs, we have empirically documented the Griffiths singularity, as exemplified by CeRhSn, which exhibits non-Fermi-liquid characteristics in susceptibility and specific heat. Our numerical analysis has supported the Griffiths phase scenario for CeRhSn and has revealed that its dc magnetic susceptibility is strongly dependent on the size of inhomogeneous magnetic particles that form in these materials. In the presence of strong disorder, we have proposed a magnetic phase diagram for CeRhSn. The classical Griffiths phase has been identified in the temperature range below the onset temperature of $T_G$ ~ 220 K, while the quantum Griffiths phase with non-Fermi liquid behavior emerges below the quantum critical temperature of $T_Q$ ~ 6 K. The phase diagram developed in this study bears notable similarities to the scenario previously proposed by Vojta for magnetic quantum phase transitions in disordered metals.

11 pages, 10 figures

References in corpus (12)

• Non-Fermi liquid behavior and Griffiths phase in {\it f}-electron compounds
• Universally diverging Grueneisen parameter and the magnetocaloric effect close to quantum critical points
• Disorder-driven non-Fermi liquid behavior in Kondo alloys
• Non-Fermi Liquid Behavior in U and Ce Alloys: Criticality, Disorder, Dissipation, and Griffiths-McCoy singularities
• Quantum Griffiths effects and smeared phase transitions in metals: theory and experiment
• Kondo disorder: a possible route towards non-Fermi liquid behavior
• Evidence for a common physical description of non-Fermi-liquid behavior in f-electron systems
• Characteristic signatures of quantum criticality driven by geometrical frustration
• Influence of disorder on the transport properties of heavy-fermion systems
• Field-angle-resolved landscape of non-Fermi-liquid behavior in the quasi-kagome Kondo Lattice CeRhSn
• Off-stoichiometric effect on magnetic and electron transport properties of Fe${}_2$VAl${}_{1.35}$ in respect to Ni${}_2$VAl; Comparative study
• Composition induced metal-insulator quantum phase transition in the Heusler type Fe2VAl