Altermagnetism and Strain Induced Altermagnetic Transition in Cairo Pentagonal Monolayer

Abstract

Altermagnetism, a recently discovered class of magnetic order characterized by vanishing net magnetization and spin-splitting band structures, has garnered significant research attention. In this work, we introduce a novel two-dimensional system that exhibits $g$-wave altermagnetism and undergoes a strain-induced transition from $g$-wave to $d$-wave altermagnetism. This system can be realized in an unconventional monolayer Cairo pentagonal lattice, for which we present a realistic tight-binding model that incorporates both magnetic and non-magnetic sites. Furthermore, we demonstrate that non-trivial band topology can emerge in this system by breaking the symmetry that protects the spin-polarized nodal points. Finally, \emph{ab initio} calculations on several candidate materials, such as FeS${}_2$ and Nb${}_2$FeB${}_2$, which exhibit symmetry consistent with the proposed tight-binding Hamiltonian, are also presented. These findings open new avenues for exploring spintronic devices based on altermagnetic systems.