All-passive upconversion of incoherent near-infrared light at intensities down to 10${}^{-7}$ W/cm${}^2$

Abstract

Frequency upconversion, which converts low-energy photons into higher-energy ones, typically requires intense coherent illumination to drive nonlinear processes or the use of externally driven optoelectronic devices. Here, we demonstrate an upconversion system that converts low-intensity (down to ~10-7 W/cm${}^2$) incoherent near-infrared (NIR) light into the visible, reaching intensities perceptible by the human eye, without the use of any external power input. Our upconverting element is enabled by the following ingredients: (1) photon upconversion via triplet-triplet annihilation in a bulk heterojunction of the organic semiconductors Y6 and rubrene; (2) plasmonic enhancement of absorption and field intensity in the heterojunction layer; (3) collection enhancement using a dichroic thin-film assembly. To enable high-resolution imaging, the upconverting element is inserted at an intermediate image plane of a dual-wavelength telescope system, which preserves the relative directionality of rays between the incident NIR light and output visible light. Our all-passive upconversion imaging system will enable NIR imaging and sensing in low-light environments under energy constraints.

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