Single vanadium ion magnetic dopant in an individual CdTe/ZnTe quantum dot
arXiv:2409.02900 · doi:10.1103/PhysRevB.111.085428
Abstract
We present the basic properties of a new physical system: an individual V2+ ion embedded into an individual quantum dot. The system is realized utilizing molecular beam epitaxy and it is observed using a low-temperature polarization-resolved magneto-photoluminescence. The nature of the system is confirmed by observation of the excitonic lines split due to the interactions of a vanadium ion with carriers confined in a CdTe/ZnTe quantum dot. Observed data are explained by the numerical modeling which includes s,p-d exchange interaction, Zeeman splitting of the exciton and the ion, diamagnetic shift, and the presence of shear strain within the quantum dot. The fundamental state of vanadium exhibits a spin +/- 1/2 making this system a textbook localized qubit.
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References in corpus (21)
- Optical manipulation of a single Mn spin in a CdTe-based quantum dot
- Optical spin orientation of a single manganese atom in a quantum dot
- Optically probing the fine structure of a single Mn atom in an InAs quantum dot
- Designing quantum dots for solotronics
- Magnetic Ground State of an Individual Fe2+ Ion in Strained Semiconductor Nanostructure
- Brightening of dark excitons in a single quantum dot containing a single magnetic ion
- Coherent precession of an individual 5/2 spin
- Individual Cr atom in a semiconductor quantum dot: optical addressability and spin-strain coupling
- Strain induced coherent dynamics of coupled carriers and Mn spins in a quantum dot
- Optical study of electron-electron exchange interaction in CdTe/ZnTe quantum dots
- Origin of luminescence quenching in structures containing CdSe/ZnSe quantum dots with a few Mn ions
- Spin dynamics of an individual Cr atom in a semiconductor quantum dot under optical excitation
- Direct measurement of hyperfine shifts and radiofrequency manipulation of the nuclear spins in individual CdTe/ZnTe quantum dots
- Direct determination of zero-field splitting for single Co ion embedded in a CdTe/ZnTe quantum dot
- A hole-Cr nano-magnet in a semiconductor quantum dot
- Influence of non-equilibrium phonons on the spin dynamics of a single Cr atom
- Fine structure of an exciton coupled to a single Fe2+ ion in a CdSe/ZnSe quantum dot
- Coherent dynamics of a single Mn-doped quantum dot revealed by four-wave mixing spectroscopy
- Charge fluctuations of a Cr atom probed in the optical spectra of a quantum dot
- Coupling of the triplet states of a negatively charged exciton in a quantum dot with the spin of a magnetic atom
- Spin dynamics of positively charged excitons in Cr-doped quantum dots probed by resonant photoluminescence