Pressure tunable magnetic skyrmion phase in Co8Zn8Mn4 single crystals

Abstract

In a magnetic skyrmion phase, magnetic moments form vortex-like topological textures which are of both fundamental and industrial interests. In ${\hat{I}}^2$-Mn-type Co-Zn-Mn alloys, chrial magnetic skyrmions emerge above room temperature, providing a unique system for studying the skrymion physics and exploring spintronics applications. However, the magnetic skyrmion phase is typically confined in a narrow and limited temperature ($T$) and magnetic field ($H$) range. Here, we demonstrate that hydrostatic pressure can expand the skyrmion phase in the $T-H$ phase diagram of single-crystalline Co${}_8$Zn${}_8$Mn${}_4$. At ambient pressure, signatures of skyrmions are seen within $T\sim 302-308$ K and $H\sim 50-100$ Oe. Applying a moderate pressure of 6 kbar extends this range to $T\sim 300-310$ K and $H\sim 50-150$ Oe. However, further escalation of pressure to 10 kbar results in a slight contraction of the skyrmion phase. These findings underscore the sensitivity of the skyrmion phase in Co${}_8$Zn${}_8$Mn${}_4$ to external pressures, and hint at the potential of strain engineering, particularly in ${\hat{I}}^2$-Mn-type Co-Zn-Mn thin films, as a promising avenue to customize the skyrmion phase.

7 pages, 4 figures