Competition between Neel, Haldane nematic, plaquette valence bond solid, and valence bond solid phases in SU(N) analogs of square-lattice antiferromagnets
arXiv:2309.12262 · doi:10.1103/PhysRevB.109.195146
Abstract
We use stochastic series expansion (SSE) quantum Monte Carlo (QMC) methods to study the phases and transitions displayed by a class of sign-free designer Hamiltonians for SU() analogs of spin quantum antiferromagnets on the square lattice. The SU() spins are generators of the single-row two-column representation (complex conjugate of single-row two-column representation) on () sublattices of the square lattice, and the Hamiltonian is designed to explore the competition between the nearest neighbour antiferromagnetic exchange couplings and four-spin interactions that favor a plaquette-ordered valence bond solid (p-VBS) ground state. We find that this state is indeed established at large for all . For , the ground state exhibits a direct first order quantum phase transition from a small- Néel ordered antiferromagnetic state to this large- p-VBS state. The ground state at for has been previously reported to be a valence bond nematic state, dubbed the Haldane nematic in recent literature. For small nonzero and , we additionally find an unusual intermediate state in which the bond energy has a Bragg peak at wavevector with no accompanying Bragg peaks at wavevectors and . This state also appears to be metastable at , as evidenced by low temperature histograms of the Haldane nematic and order parameters. Deep in the p-VBS phase of the ground state phase diagram, we find the temperature-driven melting of the p-VBS order is in the Ashkin-Teller universality class. In this regime, we identify an interesting signature of Ashkin-Teller criticality in bond correlations at wavevector ; this is in addition to the expected critical fluctuations of the conventional p-VBS order parameter at wavevectors and .
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