Charge redistribution, charge order and plasmon in La${}_{2-x}$Sr${}_x$CuO${}_4$/La${}_2$CuO${}_4$ superlattices

Abstract

Interfacial superconductors have the potential to revolutionize electronics, quantum computing, and fundamental physics due to their enhanced superconducting properties and ability to create new types of superconductors. The emergence of superconductivity at the interface of La${}_{2-x}$Sr${}_x$CuO${}_4$/La${}_2$CuO${}_4$ (LSCO/LCO), with a T${}_c$ enhancement of $\sim$ 10 K compared to the La${}_{2-x}$Sr${}_x$CuO${}_4$ bulk single crystals, provides an exciting opportunity to study quantum phenomena in reduced dimensions. To investigate the carrier distribution and excitations in interfacial superconductors, we combine O K-edge resonant inelastic X-ray scattering and atomic-resolved scanning transmission electron microscopy measurements to study La${}_{2-x}$Sr${}_x$CuO${}_4$/La${}_2$CuO${}_4$ superlattices (x=0.15, 0.45) and bulk La${}_{1.55}$Sr${}_{0.45}$CuO${}_4$ films. We find direct evidence of charge redistribution, charge order and plasmon in LSCO/LCO superlattices. Notably, the observed behaviors of charge order and plasmon deviate from the anticipated properties of individual constituents or the average doping level of the superlattice. Instead, they conform harmoniously to the effective doping, a critical parameter governed by the T${}_c$ of interfacial superconductors.

8 pages, 5 figures