Field-Emission Resonances in Thin Metallic Films: Nonexponential Decay of the Tunneling Current as a Function of the Sample-to-Tip Distance

Abstract

Field-emission resonances (FERs) for two-dimensional Pb(111) islands grown on \mbox{Si(111)7$\times$7} surfaces were studied by low-temperature scanning tunneling microscopy and spectroscopy (STM/STS) in a broad range of tunneling conditions with both active and disabled feedback loop. These FERs exist at quantized sample-to-tip distances $Z_n^{}$ above the sample surface, where $n$ is the serial number of the FER state. By recording the trajectory of the STM tip during ramping of the bias voltage $U$ (while keeping the tunneling current $I$ fixed), we obtain the set of the $Z_n^{}$ values corresponding to local maxima in the derived $dZ/dU(U)$ spectra. This way, the continuous evolution of $Z_n^{}$ as a function of $U$ for all FERs was investigated by STS experiments with active feedback loop for different $I$. Complementing these measurements by current-distance spectroscopy at a fixed $U$, we could construct a 4-dimensional $I-U-Z-dZ/dU$ diagram, that allows us to investigate the geometric localization of the FERs above the surface. We demonstrate that (i) the difference $\delta Z_n^{}=Z_{n+1}^{}-Z_n^{}$ between neighboring FER lines in the $Z-U$ diagram is independent of $n$ for higher resonances, (ii) the $\delta Z_n^{}$ value decreases as $U$ increases; (iii) the quantized FER states lead to the \emph{periodic} variations of $\ln I$ as a function of $Z$ with periodicity $\delta Z$; (iv) the periodic variations in the $\ln I-Z$ spectra allows to estimate the absolute height of the tip above the sample surface. Our findings contribute to a deeper understanding on how the FER states affect various types of tunneling spectroscopy experiments and how they lead to a non-exponential decay of the tunneling current as a function of $Z$ at high bias voltages in the regime of quantized electron emission.

25 pages, 18 figures

References in corpus (4)

• Nanoscale probing of image-potential states and electron transfer doping in borophene polymorphs
• Quantum-well and modified image-potential states in thin Pb(111) films: an estimate for the local work function
• Tunneling interferometry and measurement of thickness of ultrathin metallic Pb(111) films
• Observation of hidden parts of dislocation loops in thin Pb films by means of scanning tunneling spectroscopy

Cited by in corpus (1)

• Oscillatory Bias Dependence of Visible Height of Monatomic Pb(111) Steps: Consequence of Quantum-Size Effect for Thin Metallic Films