Room-temperature exceptional-point-driven polariton lasing from perovskite metasurface

Abstract

Excitons in lead bromide perovskites exhibit high binding energy and high oscillator strength, allowing for a strong light-matter coupling regime in the perovskite-based cavities localizing photons at the nanoscale. This opens up the way for the realization of exciton-polariton Bose-Einstein condensation and polariton lasing at room temperature -- the inversion-free low-threshold stimulated emission. However, polariton lasing in perovskite planar photon cavities without Bragg mirrors has not yet been observed and proved experimentally. In this work, we employ perovskite metasurface, fabricated with nanoimprint lithography, supporting so-called exceptional points to demonstrate the room-temperature polariton lasing. The exceptional points in exciton-polariton dispersion of the metasurface appear upon optically pumping in the nonlinear regime in the spectral vicinity of a symmetry-protected bound state in the continuum providing high mode confinement with the enhanced local density of states beneficial for polariton condensation. The observed lasing emission possesses high directivity with a divergence angle of around 1${}^{\circ }$ over one axis. The employed nanoimprinting approach for solution-processable large-scale polariton lasers is compatible with various planar photonic platforms suitable for on-chip integration.

12 pages, 3 figures

References in corpus (6)

• Polariton Bose-Einstein condensate from a Bound State in the Continuum
• Light stops at exceptional points
• Realization of room temperature polaritonic vortex in momentum space with hybrid Perovskite metasurface
• Unveiling the Enhancement of Spontaneous Emission at Exceptional Points
• Polaron-enhanced polariton nonlinearity in lead halide perovskites
• Electrically pumped polarized exciton-polaritons in a halide perovskite microcavity

Cited by in corpus (5)

• Non-Hermitian polariton-photon coupling in a perovskite open microcavity
• Mechanical scanning probe lithography of perovskites for fabrication of high-Q planar polaritonic cavities
• Magneto-Optics of Anisotropic Exciton Polaritons in Two-Dimensional Perovskites
• Identifying Exceptional Points in Two-Dimensional Excitons Coupled to an Open Optical Cavity
• Transverse instability of hybrid solitons in the strong light-matter coupling regime