paper

Localized Nitrogen-Vacancy centers generated by low-repetition rate fs-laser pulses

arXiv:2210.08071 · doi:10.1016/j.diamond.2022.109426

Abstract

Among hundreds of impurities and defects in diamond, the nitrogen-vacancy (NV) center is one of the most interesting to be used as a platform for quantum technologies and nanosensing. Traditionally, synthetic diamond is irradiated with high-energy electrons or nitrogen ions to generate these color-centers. For precise positioning of the NV centers, fs-laser irradiation has been proposed as an alternative approach to produce spatially localized NV centers in diamond. However, most of the studies reported so far used high-repetition rate fs-laser systems. Here, we studied the influence of the irradiation conditions on the generation of NV. Specifically, we varied pulse fluence, laser focusing, and the number of pulses upon irradiation with 150 fs pulses at 775 nm from a Ti:sapphire laser amplifier operating at 1 kHz repetition rate. Optically Detected Magnetic Resonance (ODMR) was used to investigate the produced NV centers, revealing a sizeable zero-field splitting in the spectra and indicating the conditions in which the lattice strain produced in the ablation process may be deleterious for quantum information applications.

15 pages, 6 figures

References in corpus (6)