Elasticity, Facilitation and Dynamic Heterogeneity in Glass-Forming liquids
arXiv:2209.08861 · doi:10.1103/PhysRevLett.130.138201
Abstract
We study the role of elasticity-induced facilitation on the dynamics of glass-forming liquids by a coarse-grained two-dimensional model in which local relaxation events, taking place by thermal activation, can trigger new relaxations by long-range elastically-mediated interactions. By simulations and an analytical theory, we show that the model reproduces the main salient facts associated with dynamic heterogeneity and offers a mechanism to explain the emergence of dynamical correlations at the glass transition. We also discuss how it can be generalized and combined with current theories.
Letter + SI
References in corpus (21)
- Theoretical perspective on the glass transition and amorphous materials
- Glassy dynamics of kinetically constrained models
- Scaling description of the yielding transition in soft amorphous solids at zero temperature
- Spatial correlations in the dynamics of glassforming liquids: Experimental determination of their temperature dependence
- Thirty milliseconds in the life of a supercooled liquid
- Relaxation in yield stress systems through elastically interacting activated events
- Microscopic origin of excess wings in relaxation spectra of supercooled liquids
- On the relevance of disorder in athermal amorphous materials under shear
- Common mechanism of thermodynamic and mechanical origin for ageing and crystallisation of glasses
- Emergence of long-ranged stress correlations at the liquid to glass transition
- Elastoplasticity Mediates Dynamical Heterogeneity Below the Mode-Coupling Temperature
- Relevance of Shear Transformations in the Relaxation of Supercooled Liquids
- Relaxation dynamics in the energy landscape of glass-forming liquids
- Fragility in Glassy Liquids: A Structural Approach Based on Machine Learning
- Finite-disorder critical point in the yielding transition of elasto-plastic models
- Thermally activated flow in models of amorphous solids
- The yielding of amorphous solids at finite temperatures
- Excess wings and asymmetric relaxation spectra in a facilitated trap model
- A Theory of Localized Excitations in Supercooled Liquids
- Mean-field description for the architecture of low-energy excitations in glasses
- Local Plastic Response and Slow Heterogeneous Dynamics of Supercooled Liquids
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- Solid-that-flows picture of glass-forming liquids
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- Unified percolation scenario for the and processes in simple glass formers
- Logarithmic aging via instability cascades in disordered systems
- Scaling Description of Dynamical Heterogeneity and Avalanches of Relaxation in Glass-Forming Liquids
- Molecular hydrodynamic theory of the velocity autocorrelation function
- Direct numerical analysis of dynamic facilitation in glass-forming liquids
- Yielding is an absorbing phase transition with vanishing critical fluctuations
- Testing theories of the glass transition with the same liquid, but many kinetic rules
- Selecting Relevant Structural Features for Glassy Dynamics by Information Imbalance
- Earthquake-like dynamics in ultrathin magnetic film
- Temperature dependence of fast relaxation processes in amorphous materials
- Ductile and brittle yielding of athermal amorphous solids: a mean-field paradigm beyond the random field Ising model
- Connecting Shear Thinning and Dynamic Heterogeneity in Supercooled Liquids by Localized Elasticity
- Starting from the amorphous ground state: linking landscape thermodynamics to slow dynamics and crossover
- General Two-Parameter Model of Alpha-Relaxation in Glasses
- Replica Field Theory for a Generalized Franz--Parisi Potential of Inhomogeneous Glassy Systems: New Closure and the Associated Self-Consistent Equation
- Rare Trajectories in a Prototypical Mean-field Disordered Model: Insights into Landscape and Instantons
- Understanding Flow Behaviors of Supercooled Liquids by Embodying Solid-Liquid Duality at Particle Level
- Cell divisions imprint long lasting elastic strain fields in epithelial tissues
- Microscopic Theory of a Fluctuation-Induced Dynamical Crossover in Supercooled Liquids
- Yielding in dense active matter