Topology of vibrational modes predict plastic events in glasses
arXiv:2209.02937 · doi:10.1038/s41467-023-38547-w
Abstract
The plastic deformation of crystalline materials can be understood by considering their structural defects such as disclinations and dislocations. Although glasses are also solids, their structure resembles closely the one of a liquid and hence the concept of structural defects becomes ill-defined. As a consequence it is very challenging to rationalize on a microscopic level the mechanical properties of glasses close to the yielding point and to relate plastic events with structural properties. Here we investigate the topological characteristics of the eigenvector field of the vibrational excitations of a two-dimensional glass model, notably the geometric arrangement of the topological defects as a function of vibrational frequency. We find that if the system is subjected to a quasistatic shear, the location of the resulting plastic events correlate strongly with the topological defects that have a negative charge. Our results provide thus a direct link between the structure of glasses prior their deformation and the plastic events during deformation.
References in corpus (10)
- Irreversible reorganization in a supercooled liquid originates from localised soft modes
- The Relationship Between Local Structure and Relaxation in Out-of-Equilibrium Glassy Systems
- Heterogeneous Dynamics, Marginal Stability and Soft Modes in Hard Sphere Glasses
- Low-energy quasilocalized excitations in structural glasses
- Predicting plasticity with soft vibrational modes: from dislocations to glasses
- Transitions among crystal, glass, and liquid in a binary mixture with changing particle size ratio and temperature
- Predicting the failure of two-dimensional silica glasses
- Elementary plastic events in amorphous silica
- Anisotropic Structural Predictor in Glassy Materials
- Correlation between plastic rearrangements and local structure in a cyclically driven glass
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- Solid-that-flows picture of glass-forming liquids
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- Experimental identification of topological defects in 2D colloidal glass
- Topological defects reveal the plasticity of glasses
- Clustering of negative topological charge precedes plastic failure in 3D glasses
- Stringlet Excitation Model of the Boson Peak
- Complete mathematical theory of the jamming transition: A perspective
- Unveiling the Asymmetry in Density within the Shear Bands of Metallic Glasses
- Phonons in stringlet-land and the boson peak
- Selecting Relevant Structural Features for Glassy Dynamics by Information Imbalance
- Properties of stable ensembles of Euclidean random matrices
- Structure-driven phase transitions in paracrystalline topological insulators
- Revealing the Geometrical and Vibrational Properties of the Defects Driving the Boson Peak
- Hedgehog topological defects in 3D amorphous solids
- Topological signatures of collective dynamics and turbulent-like energy cascades in apolar active granular
- Geometric indicators of local plasticity in glasses measured by scanning small-beam diffraction
- Graph-Dynamics correspondence in metallic glass-forming liquids
- Spotting structural defects in crystals from the topology of vibrational modes
- Emblems of pair density waves: dual identity of topological defects and their transport signatures
- Interpretability of linear regression models of glassy dynamics