Polarization dependent photoemission as a probe of the magnetic ground state in the layered ferromagnet VI3
arXiv:2206.07233 · doi:10.1063/5.0108498
Abstract
Layered ferromagnets are thrilling materials from both a fundamental and technological point of view. VI3 is an interesting example, with a complex magnetism that differentiates it from the first reported Cr based layered ferromagnets. Here, we show in an indirect way through Angle Resolved Photoemission Spectroscopy (ARPES) experiments, the importance of spin-orbit coupling setting the electronic properties of this material. Our light polarized photoemission measurements point to a ground state with a half-filled e'_+- doublet, where a gap opening is triggered by spin-orbit coupling enhanced by electronic correlations.
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- Symmetry breaking in vanadium trihalides
- Multicomponent magneto-orbital order and magneto-orbitons in monolayer VCl3
- Evidence of temperature-dependent interplay between spin and orbital moment in van der Waals ferromagnet VI3