All-electron many-body approach to resonant inelastic x-ray scattering

Abstract

We present a formalism for the resonant inelastic x-ray scattering (RIXS) cross section. The resulting compact expression in terms of polarizability matrix elements, particularly lends itself to the implementation in an all-electron many-body perturbation theory (MBPT) framework, which is realized in the full-potential package exciting. With the carbon K edge RIXS of diamond and the oxygen K edge RIXS of $\beta -\mathrm{G}{\mathrm{a}}_2{\mathrm{O}}_3$, respectively, we demonstrate the importance of electron-hole correlation and atomic coherence in the RIXS spectra.

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Cited by in corpus (1)

• Pseudopotential Bethe-Salpeter calculations for shallow-core x-ray absorption near-edge structures: excitonic effects in Al2O3