High-harmonic generation in a strongly overdriven regime

Abstract

High-harmonic generation (HHG) normally requires a careful adjustment of the driving laser intensity (typically $10^{14}-10^{15}$ W/cm${}^2$) and gas medium parameters to enable good phase matching conditions. In contrast with conventional wisdom, we present experimental results indicating phase-matched HHG in all rare gases, using a high-density medium and a driver laser intensity of around $10^{16}$ W/cm${}^2$. The experimental results are corroborated by theoretical simulations, which indicate that ionization-induced self-phase modulation and plasma defocusing self-regulate the driver laser intensity to a level that is appropriate for good phase matching. A ten-fold broadening of the NIR spectrum is observed, which results in the generation of continuous spectra from $18-140$ eV in spite of using 50-fs-long driving pulses. The presented scheme represents a simple and versatile concept for the generation of XUV and soft X-ray continua, which are ideally suited for transient absorption and reflection spectroscopy.

5 pages, 5 figures

References in corpus (6)

• Bright Coherent Ultrahigh Harmonics in the keV X-Ray Regime from Mid-Infrared Femtosecond Lasers
• Compact intense extreme-ultraviolet source
• XUV Spectral Compression by Four-Wave Mixing
• Propagation-assisted generation of intense few-femtosecond high-harmonic pulses
• The effect of plasma-core induced self-guiding on phase matching of high-order harmonic generation in gases
• Extended model for optimizing high-order harmonic generation in absorbing gases