Directing Monolayer Tungsten Disulfide Photoluminescence using a Bent Plasmonic Nanowire on a Mirror Cavity
arXiv:2203.00391 · doi:10.1140/epjs/s11734-022-00511-y
Abstract
Designing directional optical antennas without compromising the field enhancement requires specially designed optical cavities. Herein, we report on the experimental observations of directional photoluminescence emission from a monolayer Tungsten Disulfide using a bent-plasmonic nanowire on a mirror cavity. The geometry provides field enhancement and directivity to photoluminescence by sandwiching the monolayer between an extended cavity formed by dropcasting bent silver nanowire and a gold mirror. We image the photoluminescence emission wavevectors by using the Fourier plane imaging technique. The cavity out-couples the emission in a narrow range of wavevectors with a radial and azimuthal spreading of only 11.0° and 25.1°, respectively. Furthermore, we performed three dimensional finite difference time domain based numerical calculations to corroborate and understand the experimental results. We envisage that the results presented here will be readily harnessed for on-chip coupling applications and in designing inelastic optical antennas.
References in corpus (16)
- Atomically thin MoS2: A new direct-gap semiconductor
- Coupled spin and valley physics in monolayers of MoS2 and other group-VI dichalcogenides
- Control of valley polarization in monolayer MoS2 by optical helicity
- Valley polarization in MoS2 monolayers by optical pumping
- Tightly bound excitons in monolayer WSe2
- Observation of Intense Second Harmonic Generation from MoS Atomic Crystals
- Magnetic brightening and control of dark excitons in monolayer WSe2
- Strong-coupling of WSe2 in ultra-compact plasmonic nanocavities at room temperature
- In-plane Propagation of Light in Transition Metal Dichalcogenide Monolayers: Optical Selection Rules
- Helicity resolved Raman scattering of MoS2, MoSe2, WS2 and WSe2 atomic layers
- Nanoscale chiral valley-photon interface through optical spin-orbit coupling
- Comparative analysis of imaging configurations and objectives for Fourier microscopy
- Spin-orbit coupling induced valley Hall effects in transition-metal dichalcogenides
- Selective amplification of primary exciton in monolayer MoS2
- Fourier plane optical microscopy and spectroscopy
- Directional emission from WS2 monolayer coupled to plasmonic Nanowire-on-Mirror Cavity