paper

Ferroelectric control of magnetic skyrmions in two-dimensional van der Waals heterostructures

arXiv:2202.11348 · doi:10.1021/acs.nanolett.2c00564

Abstract

Magnetic skyrmions are chiral nanoscale spin textures which are usually induced by Dzyaloshinskii-Moriya interaction (DMI). Recently, magnetic skyrmions have been observed in two-dimensional (2D) van der Waals (vdW) ferromagnetic materials, such as FeGeTe. The electric control of skyrmions is important for their potential application in low-power memory technologies. Here, we predict that DMI and magnetic skyrmions in a FeGeTe monolayer can be controlled by ferroelectric polarization of an adjacent 2D vdW ferroelectric InSe. Based on density functional theory and atomistic spin-dynamics modeling, we find that the interfacial symmetry breaking produces a sizable DMI in a FeGeTe/InSe vdW heterostructure. We show that the magnitude of DMI can be controlled by ferroe-lectric polarization reversal, leading to creation and annihilation of skyrmions. Furthermore, we find that the sign of DMI in a InSe/FeGeTe/InSe heterostructure changes with ferroelectric switching reversing the skyrmion chirality. The predicted electrically controlled skyrmion formation may be interesting for spintronic applications.

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