Thermodynamics of the spin-half square-kagome lattice antiferromagnet

Abstract

Over the last decade, the interest in the spin-$1/2$ Heisenberg antiferromagnet (HAF) on the square-kagome (also called shuriken) lattice has been growing as a model system of quantum magnetism with a quantum paramagnetic ground state, flat-band physics near the saturation field, and quantum scars. Here, we present large-scale numerical investigations of the specific heat $C(T)$, the entropy $S(T)$ as well as the susceptibility $\chi (T)$ by means of the finite-temperature Lanczos method for system sizes of $N=18,24,30,36,42,48$, and $N=54$. We find that the specific heat exhibits a low-temperature shoulder below the major maximum which can be attributed to low-lying singlet excitations filling the singlet-triplet gap, which is significantly larger than the singlet-singlet gap. This observation is further supported by the behavior of the entropy $S(T)$, where a change in the curvature is present just at about $T/J=0.2$, the same temperature where the shoulder in $C$ sets in. For the susceptibility the low-lying singlet excitations are irrelevant, and the singlet-triplet gap leads to an exponentially activated low-temperature behavior. The maximum in $\chi (T)$ is found at a pretty low temperature $T_{\max }/J=0.146$ (for $N=42$) compared to $T_{\max }/J=0.935$ for the unfrustrated square-lattice HAF signaling the crucial role of frustration also for the susceptibility. We find a striking similarity of our square-kagome data with the corresponding ones for the kagome HAF down to very low $T$. The magnetization process featuring plateaus and jumps and the field dependence of the specific heat that exhibits characteristic peculiarities attributed to the existence of a flat one-magnon band are as well discussed.

11 pages, 11 figures, version as published in Phys. Rev. B

References in corpus (9)

• Strongly correlated flat-band systems: The route from Heisenberg spins to Hubbard electrons
• Magnetization plateaus in frustrated antiferromagnetic quantum spin models
• Exact low-temperature behavior of kagome antiferromagnet at high fields
• Universal low-temperature behavior of frustrated quantum antiferromagnets in the vicinity of the saturation field
• Frustrated two dimensional quantum magnets
• Universal properties of highly frustrated quantum magnets in strong magnetic fields
• Accuracy of the finite-temperature Lanczos method compared to simple typicality-based estimates
• Pinwheel valence-bond-crystal ground state of the spin-$\frac{1}{2}$ Heisenberg antiferromagnet on the $shuriken$ lattice
• Finite-temperature properties of the Kitaev-Heisenberg models on kagome and triangular lattices studied by improved finite-temperature Lanczos methods

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