Non-adiabatic Strong Field Ionization of Atomic Hydrogen
arXiv:2107.13844 · doi:10.1103/PhysRevLett.127.273201
Abstract
We present experimental data on the non-adiabatic strong field ionization of atomic hydrogen using elliptically polarized femtosecond laser pulses at a central wavelength of 390 nm. Our measured results are in very good agreement with a numerical solution of the time-dependent Schrödinger equation (TDSE). Experiment and TDSE show four above-threshold ionization (ATI) peaks in the electron's energy spectrum. The most probable emission angle (also known as 'attoclock-offset angle' or 'streaking angle') is found to increase with energy, a trend that is opposite to standard predictions based on Coulomb interaction with the ion. We show that this increase of deflection-angle can be explained by a model that includes non-adiabatic corrections of the initial momentum distribution at the tunnel exit and non-adiabatic corrections of the tunnel exit position itself.
arXiv comment8 pages, 5 figures
References in corpus (16)
- Experimental evidence for Wigner's tunneling time
- Intracycle and Intercycle Interferences in Above-Threshold Ionization: the Time Grating
- Strong Field Approximation for Systems with Coulomb Interaction
- Semiclassical two-step model for strong-field ionization
- Ultrafast Preparation and Detection of Ring Currents in Single Atoms
- Tunneling dynamics in multiphoton ionization and attoclock calibration
- Non-adiabatic Coulomb effects in strong field ionisation in circularly polarised laser fields
- Attoclock revisited on electron tunnelling time
- Direct Experimental Access to the Nonadiabatic Initial Momentum Offset upon Tunnel Ionization
- The attoclock and the tunnelling time debate
- Keldysh-Rutherford model for attoclock
- Sub-Cycle Interference upon Tunnel-Ionization by Counterrotating Two-Color Fields
- Gouy's Phase Anomaly in Electron Waves Produced by Strong-Field Ionization
- Signatures of electronic structure in bi-circular high-harmonic spectroscopy
- The cross-over from tunnelling to multiphoton ionization of atoms
- Decoding electron tunnelling delay time by embracing wave-particle duality