Generating high density molecular jets of complex neutral organic molecules using micro-sized Tesla valves

Abstract

We report the design and implementation of multiple Tesla type micro valves in the target delivery system of a reaction microscope (ReMi) to study gas phase structural dynamics of complex polyatomic molecules, when no delivery system currently exists that can deliver dense enough molecular jets of neutral complex molecules without ionizing or exciting the target. We show, the Tesla valves provide an efficient unidirectional flow of the cis-stilbene molecules into the ReMi. We demonstrate using a bubbler with Tesla valves an order-of-magnitude increase in the detected stilbene molecular ion signal following the strong-field tunnel ionization (SFTI), compared to conventional bubbler without any Tesla valves. Our results for the first time, opens the door for studying large, complex neutral molecules in the gas-phase with low vapour pressures in future ultrafast studies.

References in corpus (6)

• Laser-induced alignment and orientation of quantum-state-selected large molecules
• Observation of Quantum Effects in sub Kelvin Cold Reactions
• Symphony on Strong Field Approximation
• Quantum-state resolved bimolecular collisions of velocity-controlled OH with NO radicals
• Control and femtosecond time-resolved imaging of torsion in a chiral molecule
• Imaging an isolated water molecule using a single electron wave packet