Resonant control of photoelectron directionality by interfering one- and two-photon pathways

Abstract

Coherent control of interfering one- and two-photon processes has for decades been the subject of research to achieve the redirection of photocurrent. The present study develops two-pathway coherent control of ground state helium atom above-threshold photoionization for energies up to the $N=2$ threshold, based on a multichannel quantum defect and R-matrix calculation. Three parameters are controlled in our treatment: the optical interference phase $\Delta \Phi$, the reduced electric field strength $\chi ={\mathcal{E}}_{\omega }^2/{\mathcal{E}}_{2\omega }$, and the final state energy $\epsilon$. A small energy change near a resonance is shown to flip the emission direction of photoelectrons with high efficiency, through an example where $90\%$ of photoelectrons whose energy is near the $2p^2{}^1{S}^e$ resonance flip their emission direction. However, the large fraction of photoelectrons ionized at the intermediate state energy, which are not influenced by the optical control, make this control scheme challenging to realize experimentally.

arXiv comment5 pages, 4 figures

References in corpus (5)

• Two-color coherent control of femtosecond above-threshold photoemission from a tungsten nanotip
• A new method for measuring angle-resolved phases in photoemission
• Coherent control of population transfer between vibrational states in an optical lattice via two-path quantum interference
• One- and two-photon ionization cross sections of the laser excited 6s6p^1P_1 state of barium
• Two-photon Above Threshold Ionization of Helium

Cited by in corpus (2)

• Multichannel photoelectron phase lag across atomic barium autoionizing resonances
• Coherent control phase lag across doubly-excited atomic strontium resonances in an $\omega -2\omega$ interference scheme