Topological Surface Superconductivity Induced by Hydrostatic Pressure-Enhanced Antisymmetric Spin-Orbit Coupling in Non-Centrosymmetric Superconductor PbTaSe2

Abstract

A notable characteristic of PbTaSe${}_2$, a prototypical noncentrosymmetric (NCS) superconductor, is that its superconductivity can be modulated through a structural transition under hydrostatic pressure [Phys. Rev. B 95, 224508 (2017)]. Here we report on simultaneous pressure-sensitive point-contact Andreev reflection (PCAR) spectroscopy and bulk resistance measurements on PbTaSe${}_2$, to elucidate the nature of the surface and bulk superconductivity and their evolution with hydrostatic pressure. It is found that in high pressure region the superconducting gap opening temperature $T_c^A$ is significantly lower that the bulk resistive transition temperature $T_c^R$, revealing a clear experimental signature of surface-bulk separation associated with enhanced antisymmetric spin-orbit coupling (ASOC). The PCAR spectra, reflecting the superconducting surface state, are analyzed with the Blonder-Tinkham-Klapwijk theory, yielding an isotropic $s$-wave full BCS-gap in the strong coupling regime. Analysis based on a modified McMillan formula indicates a sizable coupling strength contributed from ASOC for the superconducting surface state. These results suggest the coexistence of full gap $s$-wave superconductivity and topological surface states in PbTaSe${}_2$, indicating that this NSC with significantly enhanced ASOC may offer a solid platform to investigate the topological aspect in the superconducting condensate.

References in corpus (8)

• Superconducting proximity effect and Majorana fermions at the surface of a topological insulator
• Majorana Fermions and a Topological Phase Transition in Semiconductor-Superconductor Heterostructures
• Classification of topological insulators and superconductors in three spatial dimensions
• Topological Phases of Noncentrosymmetric Superconductors: Edge States, Majorana Fermions, and the Non-Abelian Statistics
• Evidence for time-reversal symmetry breaking in the non-centrosymmetric superconductor LaNiC${}_2$
• Dirac Surface States and Nature of Superconductivity in Noncentrosymmetric BiPd
• Surface bound states and spin currents in non-centrosymmetric superconductors
• Abrupt enhancement of non-centrosymmetry and appearance of the spin-triplet superconducting state in Li_2(Pd_{1-x}Pt_{x})_3B beyond x=0.8