Successive destruction of charge density wave states by pressure in LaAgSb${}_2$

Abstract

We comprehensively studied the magnetotransport properties of LaAgSb${}_2$ under high pressure up to 4 GPa, which showed unique successive charge density wave (CDW) transitions at $T_{CDW1}\sim 210$ K and $T_{CDW2}\sim 190$ K at ambient pressure. With the application of pressure, both $T_{CDW1}$ and $T_{CDW2}$ were suppressed and disappeared at the critical pressures of $P_{CDW1}=3.0$--3.4 GPa and $P_{CDW2}=1.5$--1.9 GPa, respectively. At $P_{CDW1}$, the Hall conductivity showed a step-like increase, which is consistently understood by the emergence of two-dimensional hollow Fermi surface at $P_{CDW1}$. We also observed a significant negative magnetoresistance effect when the magnetic field and current were applied parallel to the $c$ axis. Shubnikov--de Haas (SdH) oscillation measurements under pressure directly showed the changes in the Fermi surface across the CDW phase boundaries. In $P<P_{CDW2}$, three major oscillation components, $\alpha$, $\beta$, and $\gamma$, were identified, whose frequencies were increased by application of pressure. The increment rate of these frequencies was considerably larger than that expected from the shrinkage of lattice constant, indicating the unignorable band modification under pressure. In the normal metallic phase above $P>P_{CDW1}$, we observed a single frequency of $\sim 48$ T with a cyclotron effective mass of 0.066 $m_0$, whose cross section in the reciprocal space corresponded to only 0.22\% of the first Brillouin zone. Besides, we observed another oscillation component with frequency of $\sim 9.2$ T, which is significantly enhanced in the limited pressure range of $P_{CDW2}<P<P_{CDW1}$. The amplitude of this oscillation was anomalously suppressed in the high-field and low-temperature region, which cannot be explained by the conventional Lifshitz--Kosevich formula.

arXiv comment15pages, 13 figures

References in corpus (16)

• Topological Insulator Materials
• Chiral Anomaly and Classical Negative Magnetoresistance of Weyl Metals
• Negative magnetoresistance without well-defined chirality in the Weyl semimetal TaP
• Fermi surface nesting and the origin of Charge Density Waves in metals
• On the search for the chiral anomaly in Weyl semimetals: The negative longitudinal magnetoresistance
• Alternative route to charge density wave formation in multiband systems
• Multiband effects and the possible Dirac states in LaAgSb${}_2$
• Observation of Dirac-like band dispersion in LaAgSb${}_2$
• Origin of the large anisotropic g-factor of holes in bismuth
• Dirac Fermions and Possible Weak Antilocalization in LaCuSb${}_2$
• Hydrostatic pressure study of pure and doped La1-xRxAgSb2 (R = Ce, Nd) charge-density-wave compounds
• Thermal expansion and magnetostriction of pure and doped RAgSb2 (R = Y, Sm, La) single crystals
• Quantitative evaluation of Dirac physics in PbTe
• Crystalline spin-orbit interaction and the Zeeman splitting in Pb${}_{1-x}$Sn${}_x$Te
• Tuning of charge density wave transitions in LaAu${}_x$Sb${}_2$ by pressure and Au-stoichiometry
• Longitudinal and transverse magnetoresistance of SrTiO${}_3$ with a single closed Fermi surface

Cited by in corpus (5)

• Electronic band structure and surface states in Dirac semimetal LaAgSb${}_2$
• Observation of superconductivity and its enhancement at the charge density wave critical point in LaAgSb${}_2$
• Magnetotransport studies of the Sb square-net compound LaAgSb${}_2$ under high pressure and rotating magnetic fields
• Phonon-mediated superconductivity in the Sb-square-net compound LaCuSb${}_2$
• Effects of physical and chemical pressure on charge density wave transitions in LaAg1-xAuxSb2 single crystals