Femtosecond currents in transition metal dichalcogenides monolayers

Abstract

We theoretically study the interaction of an ultrafast intense linearly polarized optical pulse with monolayers of transition metal dichalcogenides (TMDCs). Such a strong pulse redistributes electrons between the bands and generates femtosecond currents during the pulse. Due to the large bandwidth of the incident pulse, this process is completely off-resonant. While in TMDCs the time-reversal symmetry is conserved, the inversion symmetry is broken and these monolayers have the axial symmetry along armchair direction but not along the zigzag one. Therefore, the pulse polarized along the asymmetric direction of TMDC monolayer generates both longitudinal, i.e., along the direction of polarization, and transverse, i.e., in the perpendicular direction, currents. Such currents result in charge transfer through the system. We study different TMDC materials and show how the femtosecond transport in TMDC monolayers depend on their parameters, such as lattice constant and bandgap.

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