Three interaction energy scales in single-layer high-T${}_C$ cuprate HgBa${}_2$CuO${}_{4+\delta }$

Abstract

The lamellar cuprate superconductors exhibit the highest ambient-pressure superconducting transition temperatures (T${}_C$) and, after more than three decades of extraordinary research activity, continue to pose formidable scientific challenges. A major experimental obstacle has been to distinguish universal phenomena from materials- or technique-dependent ones. Angle-resolved photoemission spectroscopy (ARPES) measures momentum-dependent single-particle electronic excitations and has been invaluable in the endeavor to determine the anisotropic momentum-space properties of the cuprates. HgBa${}_2$CuO${}_{4+\delta }$ (Hg1201) is a single-CuO${}_2$-layer cuprate with a particularly high optimal T${}_C$ and a simple crystal structure; yet there exists little information from ARPES about the electronic properties of this model system. Here we present an ARPES study of doping-, temperature-, and momentum-dependent systematics of near-nodal dispersion anomalies in Hg1201. The data reveal a hierarchy of three distinct energy scales -a sub-gap low-energy kink, an intermediate-energy kink near 55 meV, and a peak-dip-hump structure. The first two features are attributed to the coupling of electrons to Ba-derived optical phonons and in-plane bond-stretching phonons, respectively. The nodal peak-dip-hump structure appears to have a common doping-dependence in several single-layer cuprates, and is interpreted as a manifestation of pseudogap physics at the node. These results establish several universal phenomena, both in terms of connecting multiple experimental techniques for a single material, and in terms of connecting comparable spectral features in multiple structurally similar cuprates.

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Cited by in corpus (7)

• Constrained-Path Auxiliary-Field Quantum Monte Carlo for Coupled Electrons and Phonons
• Superconducting critical temperature in the extended diffusive SYK model
• Extracting correlation effects from Momentum-Resolved Electron Energy Loss Spectroscopy (M-EELS): Synergistic origin of the dispersion kink in Bi${}_{2.1}$Sr${}_{1.9}$CaCu${}_2$O${}_{8+x}$
• Enhanced superconducting gap in the outer CuO${}_2$ plane of the trilayer cuprate (Hg,Re)Ba${}_2$Ca${}_2$Cu${}_3$O${}_{8+\delta }$
• Observation of the Yamaji effect in a cuprate superconductor
• The pseudogap in hole-doped cuprates: possible insights from the Kondo effect
• Electronic Structure and Superconducting Gap of HgBa${}_2$Ca${}_2$Cu${}_3$O${}_{8+\delta }$ Revealed by Laser-Based Angle-Resolved Photoemission Spectroscopy