Probing photo-induced rearrangements in the NdNiO${}_3$ magnetic spiral with polarization-sensitive ultrafast resonant soft x-ray scattering

Abstract

We use resonant soft X-ray diffraction to track the photo-induced dynamics of the antiferromagnetic structure in a NdNiO${}_3$ thin film. Femtosecond laser pulses with a photon energy of 0.61 eV, resonant with electron transfer between long-bond and short-bond nickel sites, are used to excite the material and drive an ultrafast insulator-metal transition. Polarization sensitive soft X-ray diffraction, resonant to the nickel L${}_3$-edge, then probes the evolution of the underlying magnetic spiral as a function of time delay with 80 picosecond time resolution. By modelling the azimuthal dependence of the scattered intensity for different linear X-ray polarizations, we benchmark the changes of the local magnetic moments and the spin alignment. The measured changes are consistent with a reduction of the long-bond site magnetic moments and an alignment of the spins towards a more collinear structure at early time delays.

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