Coupling lattice instabilities across the interface in ultrathin oxide heterostructures

Abstract

Oxide heterointerfaces constitute a rich platform for realizing novel functionalities in condensed matter. A key aspect is the strong link between structural and electronic properties, which can be modified by interfacing materials with distinct lattice symmetries. Here we determine the effect of the cubic-tetragonal distortion of ${\text{SrTiO}}_3$ on the electronic properties of thin films of ${\text{SrIrO}}_3$, a topological crystalline metal hosting a delicate interplay between spin-orbit coupling and electronic correlations. We demonstrate that below the transition temperature at 105 K, ${\text{SrIrO}}_3$ orthorhombic domains couple directly to tetragonal domains in ${\text{SrTiO}}_3$. This forces the in-phase rotational axis to lie in-plane and creates a binary domain structure in the ${\text{SrIrO}}_3$ film. The close proximity to the metal-insulator transition in ultrathin ${\text{SrIrO}}_3$ causes the individual domains to have strongly anisotropic transport properties, driven by a reduction of bandwidth along the in-phase axis. The strong structure-property relationships in perovskites make these compounds particularly suitable for static and dynamic coupling at interfaces, providing a promising route towards realizing novel functionalities in oxide heterostructures.

5 pages, 4 figures