Correlated motion of particle-hole excitations across the renormalized spin-orbit gap in $\mathrm{S}{\mathrm{r}}_2\mathrm{Ir}{\mathrm{O}}_4$

Abstract

The high-energy collective modes of particle-hole excitations across the spin-orbit gap in $\mathrm{S}{\mathrm{r}}_2\mathrm{Ir}{\mathrm{O}}_4$ are investigated using the transformed Coulomb interaction terms in the pseudo-spin-orbital basis constituted by the $J=1/2$ and $3/2$ states arising from spin-orbit coupling. With appropriate interaction strengths and renormalized spin-orbit gap, these collective modes yield two well-defined propagating spin-orbit exciton modes, with energy scale and dispersion in excellent agreement with resonant inelastic X-ray scattering (RIXS) measurements.

arXiv comment14 pages, 4 figures. arXiv admin note: substantial text overlap with arXiv:1903.03360

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Cited by in corpus (4)

• Magnetic reorientation transition in a three orbital model for $\mathrm{C}{\mathrm{a}}_2\mathrm{Ru}{\mathrm{O}}_4$ -- Interplay of spin-orbit coupling, tetragonal distortion, and Coulomb interactions
• Modeling multiorbital effects in Sr2IrO4 under strain and a Zeeman field
• Coupled spin-orbital fluctuations in a three orbital model for $4d$ and $5d$ oxides with electron fillings $n=3,4,5$ -- Application to $\mathrm{NaOs}{\mathrm{O}}_3$, $\mathrm{C}{\mathrm{a}}_2\mathrm{Ru}{\mathrm{O}}_4$, and $\mathrm{S}{\mathrm{r}}_2\mathrm{Ir}{\mathrm{O}}_4$
• Pseudo-spin rotation symmetry breaking by Coulomb interaction terms in spin-orbit coupled systems