Kondo physics of magnetic adatoms on metallic surfaces when the onset of the surface conduction density of states crosses the Fermi level
arXiv:1910.05239 · doi:10.1103/PhysRevB.100.165139
Abstract
We study the role of the onset of Shockley states, , belonging to (111) surfaces of Cu, Ag and Au in the Kondo effect when a magnetic impurity is deposited on them. When approaches to the Fermi level, , thing that can be done by compressing (stretching) the metallic sample, we found that most of the thermodynamic and dynamic properties of the impurity are affected in a non trivial way. We model the system by a generic Anderson impurity model and solve it by using the numerical renormalization group, NRG, technique. In particular, the impurity contribution to magnetic susceptibility and entropy as a function of temperature exhibit negative values and goes to zero slowly in a logarithmic shape. Furthermore, we found a suppression of the spectral density weight at the Fermi level when even in the Kondo regime. As a consequence, the conductance through the impurity is strongly reduced by near of the unitary value . Finally, we analyze these features in realistic systems like Co on Ag(111) reported in the literature.
arXiv commentaccepted in Phys. Rev. B, 11 pages, 13 figures
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