Antiferromagnetic Stacking of Ferromagnetic Layers and Doping Controlled Phase Competition in CaSrCoAs
arXiv:1904.06444 · doi:10.1103/PhysRevB.100.024415
Abstract
In search of a quantum phase transition between the two-dimensional (D) ferromagnetism of CaCoAs and stripe-type antiferromagnetism in SrCoAs, we rather find evidence for D magnetic frustration between magnetic square Co layers. We present neutron diffraction data for CaSrCoAs that reveal a sequence of -dependent magnetic transitions which involve different stacking of D ferromagnetically-aligned layers with different magnetic anisotropy. We explain the -dependent changes to the magnetic order by utilizing classical analytical calculations of a D Heisenberg model where single-ion magnetic anisotropy and frustration of antiferromagnetic nearest- and next-nearest-layer exchange are all composition dependent.
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