paper

Complex exchange mechanism driven ferromagnetism in half-metallic Heusler CoTiGe: Evidence from critical behavior

arXiv:1903.10987 · doi:10.1103/PhysRevB.99.214414

Abstract

We have investigated the critical phenomenon associated with the magnetic phase transition in the half-metallic full-Heusler CoTiGe. The compound undergoes a continuous ferromagnetic to paramagnetic phase transition at the Curie temperature =371.5 K. The analysis of magnetization isotherms in the vicinity of , following modified Arrott plot method, Kouvel-Fisher technique, and critical isotherm plot, yields the asymptotic critical exponents =0.495, =1.324, and =3.67. The self-consistency and reliability of the obtained exponents are further verified by the Widom scaling relation and scaling equation of states. The mean-field-like value of the critical exponent suggests long-range nature of the exchange interactions, whereas the values of the critical exponents and , imply sizeable critical spin fluctuations. The half-metallic itinerant character of CoTiGe in the presence of magnetic inhomogeneity may result in such a strong deviation from the three-dimensional Heisenberg values (=0.369, =1.38 and =4.8) of the critical exponents towards the mean field values (=0.5, =1 and =3). The results suggest complex nature of exchange couplings that stabilize the long-range ferromagnetic ordering in the system and are consistent with the earlier theoretical studies on the exchange mechanism in CoTiGe.

9 pages, 8 figures

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