Magnetocaloric properties of frustrated tetrahedra-based spin nanoclusters
arXiv:1903.01754 · doi:10.1016/j.physleta.2019.05.015
Abstract
Magnetization, entropy and magnetocaloric properties of various geometrically frustrated tetrahedra-based Ising antiferromagnetic nanoclusters with corner-, edge-, and face-sharing topologies are studied by exact enumeration. It is found that the studied properties strongly depend on the nanocluster topology and can be very different from those of a single tetrahedron as well as the pyrochlore lattice formed by an infinite number of corner-sharing tetrahedra. From the magnetocaloric point of view an important difference from the latter two systems is the absence of the ground-state zero-magnetization plateau in most of the studied structures, which at low temperatures facilitates emergence of a giant magnetocaloric effect in a vanishing magnetic field in the adiabatic demagnetization process. Magnetic systems with such properties might be suitable candidates for technological application as efficient refrigerators to ultra-low temperatures.
16 pages, 7 figures
References in corpus (9)
- Magnetothermal properties of molecule-based materials
- Enhanced magnetocaloric effect in frustrated magnets
- Spin-enhanced magnetocaloric effect in molecular nanomagnets
- Enhanced magnetocaloric effect in frustrated magnetic molecules with icosahedral symmetry
- Magnetocaloric effect in pyrochlore antiferromagnet Gd2Ti2O7
- Non-universality of artificial frustrated spin systems
- Enhanced magnetocaloric effect in a proximity of magnetization steps and jumps of spin-1/2 XXZ Heisenberg regular polyhedra
- Thermodynamic and magnetocaloric properties of geometrically frustrated Ising nanoclusters
- Magneto-thermal properties of the spin-s Heisenberg antiferromagnet on the cuboctahedron
Cited by in corpus (4)
- Magnetocaloric properties of V6 molecular magnet
- Magnetocaloric and electrocaloric properties of the Hubbard pair cluster
- Theoretical analysis of magnetic properties and the magnetocaloric effect using the Blume-Capel model
- Enhancement of the Magnetocaloric Effect in Geometrically Frustrated Cluster Spin Glass Systems