Angle-Resolved Spectra of the Direct Above-Threshold Ionization of Diatomic Molecule in IR+XUV laser field

Abstract

The direct above-threshold ionization (ATI) of diatomic molecules in linearly-polarized infrared and extreme ultraviolet (IR+XUV) laser fields is investigated by the frequency-domain theory based on the nonperturbative quantum electrodynamics. The destructive interference fringes on the angle-resolved ATI spectra, which are closely related to the molecular structure, can be well fitted by a simple predictive formula for any alignment of the molecular axis. By comparing the direct ATI spectra for monochromatic and two-color laser fields, we found that the XUV laser field can both raise the ionization probability and the kinetic energy of the ionized electron, while the IR laser field can broaden the energy distribution of the ionized electron. Our results demonstrate that, by using IR+XUV two-color laser fields, the angle-resolved spectra of the direct ATI can image the structural information of molecules without considering the recollision process of the ionized electron.

7 figures

References in corpus (2)

• Accurate retrieval of structural information from laser-induced photoelectron and high-harmonic spectra by few-cycle laser pulses
• Interference effects in above-threshold ionization from diatomic molecules: determining the internuclear separation