Local-noise spectroscopy for non-equilibrium systems

Abstract

We introduce the notion, and develop the theory of local-noise spectroscopy (LNS) - a tool to study the properties of systems far from equilibrium by means of flux density correlations. As a test bed, we apply it to biased molecular junctions. This tool naturally extends those based on local fluxes, while providing complementary information on the system. As examples of the rich phenomenology that one can study with this approach, we show that LNS can be used to yield information on microscopic properties of bias-induced light emission in junctions, provide local resolution of intra-system interactions, and employed as a nano-thermometry tool. Although LNS may, at the moment, be difficult to realize experimentally, it can nonetheless be used as a powerful theoretical tool to infer a wide range of physical properties on a variety of systems of present interest.

7 pages, 4 figures

References in corpus (4)

• Vibrational and electronic heating in nanoscale junctions
• Theory of light emission from quantum noise in plasmonic contacts: above-threshold emission from higher-order electron-plasmon scattering
• Spin-polarized current and shot noise in the presence of spin flip in a quantum dot via nonequilibrium Green's functions
• Ab initio spin-flip conductance of hydrogenated graphene nanoribbons: Spin-orbit interaction and scattering with local impurity spins