paper

Isotopic trends of quasifission and fusion-fission in the reactions Ca+Pu

arXiv:1810.13114 · doi:10.1103/PhysRevC.98.064609

Abstract

Background: Quasifission and fusion-fission are primary mechanisms to prevent the production of superheavy elements. The recent experimental measurements reveal that the fusion-evaporation cross section in the reaction channel of Ca+Pu is 50 times lower than using Pu as target nucleus. However, the precise mechanisms of this remarkable isotopic dependence are not well understood. Purpose: To understand the experimental observation of the rapid decrease of stability of superheavy nuclei as the neutron number decreases, the theoretical studies of quasifission and fusion-fission in connection with experimental production for =114 flerovium isotopes are required to investigate the possible differences in reaction mechanisms induced by these two targets. Methods: We propose an approach called TDHF+HIVAP to take into account both the evolution of dinuclear system and the deexcitation of compound nucleus, which combines the microscopic time-dependent Hartree-Fock (TDHF) method for the fusion and quasifission dynamics with the statistical evaporation model HIVAP for fusion-fission dynamics. Results: ......The quantum shell effect displays a crucial role in both the quasifission and the fusion-fission processes. The quasifission is considerably reduced and the survival probability is enhanced around one order of magnitude in the reaction using Pu target as compared to the Pu case. Conclusions: The studies by using TDHF+HIVAP method well account for the experimental observations and the present method clearly shows its applicability in the reaction mechanisms of quasifission and fusion-fission dynamics. The experimental and theoretical results encourage the use of neutron-rich targets for the production of new superheavy elements.

10 pages, 7 figures

Isotopic trends of quasifission and fusion-fission in the reactions $^{48}$Ca+$^{239,244}$Pu · wovepaper