Hyperfine interaction and electronic spin fluctuation study on Sr${}_{2-x}$La${}_x$FeCoO${}_6$ (x = 0, 1, 2) by high-resolution back-scattering neutron spectroscopy

Abstract

The study of hyperfine interaction by high-resolution inelastic neutron scattering is not very well known compared to the other competing techniques viz. NMR, Mössbauer, PACS etc. Also the study is limited mostly to magnetically ordered systems. Here we report such study on Sr${}_{2-x}$La${}_x$FeCoO${}_6$ (x = 0, 1, 2) of which first (Sr${}_2$FeCoO${}_6$ with x = 0) has a canonical spin spin glass, the second (SrLaFeCoO${}_6$ with x = 1) has a so-called magnetic glass and the third (La${}_2$FeCoO${}_6$ with x = 2) has a magnetically ordered ground state. Our present study revealed clear inelastic signal for SrLaFeCoO${}_6$, possibly also inelastic signal for Sr${}_2$FeCoO${}_6$ below the spin freezing temperatures $T_{sf}$ but no inelastic signal at all for for the magnetically ordered La${}_2$FeCoO${}_6$ in the neutron scattering spectra. The broadened inelastic signals observed suggest hyperfine field distribution in the two disordered magnetic glassy systems and no signal for the third compound suggests no or very small hyperfine field at the Co nucleus due to Co electronic moment. For the two magnetic glassy system apart from the hyperfine signal due only to Co, we also observed electronic spin fluctuations probably from both Fe and Co electronic moments. \end{abstract}